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Τύπος: Άρθρο σε επιστημονικό περιοδικό
Τίτλος: Source apportionment of fine organic and inorganic atmospheric aerosol in an urban background area in Greece
Συγγραφέας: [EL] Μανούσακας, Μανούσος - Ιωάννης[EN] Manousakas, Manousos - Ioannissemantics logo
[EL] Φλώρου, Καλλιόπη[EN] Florou, Kalliopisemantics logo
[EL] Πανδής, Σπυρίδων[EN] Pandis, Spyrossemantics logo
Ημερομηνία: 29/03/2020
Περίληψη: Fine particulate matter (PM) originates from various emission sources and physicochemical processes. Quantification of the sources of PM is an important step during the planning of efficient mitigation strategies and the investigation of the potential risks to human health. Usually, source apportionment studies focus either on the organic or on the inorganic fraction of PM. In this study that took place in Patras, Greece, we address both PM fractions by combining measurements from a range of on- and off-line techniques, including elemental composition, organic and elemental carbon (OC and EC) measurements, and high-resolution Aerosol Mass Spectrometry (AMS) from different techniques. Six fine PM2.5 sources were identified based on the off-line measurements: secondary sulfate (34%), biomass burning (15%), exhaust traffic emissions (13%), nonexhaust traffic emissions (12%), mineral dust (10%), and sea salt (5%). The analysis of the AMS spectra quantified five factors: two oxygenated organic aerosols (OOA) factors (an OOA and a marine-related OOA, 52% of the total organic aerosols (OA)), cooking OA (COA, 11%) and two biomass burning OA (BBOA-I and BBOA-II, 37% in total) factors. The results of the two methods were synthesized, showcasing the complementarity of the two methodologies for fine PM source identification. The synthesis suggests that the contribution of biomass burning is quite robust, but that the exhaust traffic emissions are not due to local sources and may also include secondary OA from other sources.
Γλώσσα: Αγγλικά
Τόπος δημοσίευσης: Patras, Greece
Σελίδες: 17
DOI: 10.3390/atmos11040330
ISSN: 2073-4433
Θεματική κατηγορία: [EL] Μετεωρολογία και Επιστήμες της ατμόσφαιρας[EN] Meteorology and Atmospheric Sciencessemantics logo
Λέξεις-κλειδιά: source apportionmentPositive Matrix Factorization (PMF)AMSchemical composition
Κάτοχος πνευματικών δικαιωμάτων: © 2020 by the authors. Licensee MDPI
Όροι και προϋποθέσεις δικαιωμάτων: This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/)
Διατίθεται ανοιχτά στην τοποθεσία: https://www.mdpi.com/2073-4433/11/4/330
Ηλεκτρονική διεύθυνση του τεκμηρίου στον εκδότη: https://www.mdpi.com/2073-4433/11/4/330
Ηλεκτρονική διεύθυνση περιοδικού: https://www.mdpi.com/journal/atmosphere
Τίτλος πηγής δημοσίευσης: Atmosphere
Τεύχος: 4
Τόμος: 11
Σελίδες τεκμηρίου (στην πηγή): 330(1-17)
Σημειώσεις: This research was financed by the European Union and Greek national funds through the program "Support for Researchers with Emphasis on Young Researchers" (call code: EDBM34), operational program "Development of Human Resources, Education and Lifelong Learning", NSRF 2014–2020, and under the research title: "Source apportionment of fine atmospheric aerosols and their organic component in urban and regional background areas in West Greece, for assisting air pollution and climate change long term management," MIS 5005098.
(This article belongs to the Special Issue Sources and Composition of Ambient Particulate Matter)
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